Jude Law

Sky Captain

Gwyneth Paltrow

Polly Perkins

Angelina Jolie

Franky

Giovanni Ribisi

Dex

Michael Gambon

Paley

Bai Ling

Mysterious Woman

Omid Djalili

Kaji

Laurence Olivier

Dr. Totenkopf (archive footage)

Trevor Baxter

Dr Walter Jennings

Jon Rumney

German Scientist

Khan Bonfils

Creepy

Louis Hilyer

Executive Officer

Steve Morphew

Crewman #2

Nancy Crane

Receptionist

Stuart Milligan

Police Sergeant

Demetri Goritsas

Radio Operator

William Hope

American Broadcaster

Jonathan Keeble

British Broadcaster

Stéphane Cornicard

French Broadcaster

Stephen Ballantyne

German Broadcaster

Mido Hamada

Soldier

Gerard Monaco

Technician

James Bannon

Voice Actor (uncredited)

Sky Soleil

Officer (uncredited)